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Organic Chemistry

Topic 13 of 34

Cyanide attacks the carbonyl carbon, then oxygen is protonated

The carbonyl becomes a tetrahedral hydroxynitrile centre and the carbon chain gains one carbon.

A-Level 9476 (2026-2027)

Cyanide attacks the carbonyl carbon, then oxygen is protonated

The carbonyl becomes a tetrahedral hydroxynitrile centre and the carbon chain gains one carbon.

Use HCN with a small amount of KCN as catalyst. HCN alone supplies only a low concentration of CN-; the cyanide ion is the nucleophile. Its carbon end donates a lone pair to the δ+ carbonyl carbon, while the C=O π pair moves onto oxygen. Protonation of the resulting alkoxide by HCN produces the hydroxynitrile and regenerates CN-.

Nucleophilic addition to ethanal

A lone pair on the carbon end of N triple bond C minus points to the carbonyl carbon. At the same time the carbonyl pi bond points towards oxygen, producing an O-minus alkoxide rather than a carbon with five bonds.

The two arrows occur in the same addition step. Cyanide contributes a carbon atom; it is not attached through nitrogen.
Complete the mechanism and regenerate the catalyst
  1. Form the alkoxide

    CH3CHO + CN- → CH3CH(O-)CN. The negative charge is on oxygen.

  2. Transfer a proton from HCN

    The oxygen lone pair goes to H in H-CN; the H-C bond pair returns to the cyanide carbon.

  3. Write the product

    CH3CH(O-)CN + HCN → CH3CH(OH)CN + CN-. Overall, HCN adds across C=O.

An aldehyde RCHO gives RCH(OH)CN; a ketone R2CO gives R2C(OH)CN. Attack on either face of a planar carbonyl can form a racemic pair if a new chiral centre is created in an otherwise achiral system. Ethanal creates such a centre; propanone does not, because the product has two identical methyl groups.

Check your understandingWhy must an arrow move the carbonyl pi pair onto oxygen when CN- forms a new bond to carbon?Think it through, then reveal the answer
Without that movement, the carbon would exceed its usual octet. The pi pair becomes an oxygen lone pair, giving a tetrahedral alkoxide. The later protonation changes O- into OH.